Also, try using the "swapfile" parameter on the pss analysis. This allows the data captured during the shooting interval to be memory mapped to a set of files, which allows more than 4G of memory to be accessed (in effect). There was also a memory problem with higher numbers of harmonics, if my memory is correct - but I recall that being fixed in an MMSIM60 hotfix - so MMSIM61 USR1 should be a good thing to aim for.
If you have enough memory though, you could use the 64 bit version by doing:
Code:setenv CDS_AUTO_64BIT spectre
Regards,
Andrew.